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Y.on("click", function (e) {
    var url = '/GrantApplication/GetEmployeeInfo';

    Y.io(url, {
        method: "POST",
        data: {
            "employeeNumber": Y.one('#EmployeeNumber').get('value')
        },
        on: {
            success: function (id, o) {
                var data = JSON.parse(o.responseText);

                Y.one('#Title').set('value', data.Title);
                // ...
            }
        }
    }
}, '#btnPrepopulateEmployeeDetails');

      var xhr = new Y.Base.InlineXhr();
      xhr.setConfig({url: '/GrantApplication/GetEmployeeInfo', mode: 'alert', method: 'GET'});
      
      var data = { employeeNumber: Y.one('#EmployeeNumber').get('value') };      

      var employeeIO = xhr.register(employeeIO,'getEmployee',data);      

      Y.on("click", employeeIO.request, "#btnPrepopulateEmployeeDetails", employeeIO);
      
        /* you would call this function from your PHP "getEmployee()" function, method or Smarty plugin */
      Y.showEmployee = function(data){
         Y.one('#Title').set('value',data.Title);
         /* ... more data ... */
      }